"Optical spectroscopy of a GaAs/AlGaAs multiple quantum well system near double exciton-polariton and Bragg resonance" Abstract

We studied optical reflection (OR) and contactless electroreflection (CER) from a periodic system of multiple GaAs/AlGaAs quantum wells (QWs). The system was designed in such way that the electromagnetic resonance of Bragg reflection occurs at the frequency that coincides or is close to the frequency of the exciton-polariton resonance in the wells. Under these conditions there should be electromagnetic coupling between excitonic states in the QWs. Optical measurements were made at various temperatures, angles of the light incidence and polarization. The optical reflection spectra have been found to be a result of the interplay of three different contributions, namely (i) the reflection from the air/semiconductor interface, (ii) the Bragg reflection due to periodic modulation of the background indices of refraction being different for the wells and barriers and (iii) the resonant reflection from the periodic system of exciton-polaritons in quantum wells. The latter contribution was separately studied by CER technique in the spectral range covering ground states of the heavy-hole and light-hole excitons. A quantitative analysis of the experimental CER line shape has been done along with quantum-mechanical calculations, which revealed the characteristic energies and broadening parameters for different exciton-polariton levels. In particular, the systems of four and thirty two QWs exhibit spectral features with the characteristic broadening of 1.8 meV and 2.2 meV at 17 K, respectively. By comparison of the experimental data with theoretical calculations we discuss the radiative and non-radiative contributions to the total broadening.